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Here's an unfinished animation of Ash I did almost a year ago, with similar goals in mind. I gave up on this because I didn't feel I had the right level of skills, so I've really come a long way!
When doing the shadows, I made sure to draw everything in blobs and chunks to look like they were done with paint brushes.
You can see the different in coloring styles between FLCL and FLCL: Progressive.
While I'm finishing up this animation, I might as well post this unfinished one.
This the only shot I finished for a short animation test I was going to do last year, but fall finals got in the way.