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2. Ledyba
There's a fantastic scene in Breaking Bad where Jesse plays with a beetle. This is the only unevolved beetle Pokémon (Jesse is going to have mostly unevolved Pokémon) Its immature yet spirited nature fits Jesse, especially when that spirit gets crushed like a beetle.
6. Vileplume
To round out Walter's team, he has a toxic plant, one that he might use in a powder to kill his enemies or in a juice box to orchestrate a scheme.