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Richard Deakin's 1000+ unpublished watercolours of fungi show developmental stages, cross sections & microscopic views of spores, along with details of locality, date & habitat; so can function as actual biological records
Beautiful portrait of the Kentish Glory moth - male, female, and larva - from Curtis's British Entomology 1833
Great illustrated entomological books: George Buckton, Monograph of the British Aphides, 1875-82
Great Illustrated entomological books: William Fowler's British Coleoptera, 1887-91